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ryan-2022-emissions

Impact of Rocket Launch and Space Debris Air Pollutant Emissions on Stratospheric Ozone and Global Climate

Robert G. Ryan, Eloise A. Marais, Chloe J. Balhatchet, Sebastian D. Eastham 2022 paper cited by: q2-earth-atmospheric-ceiling
https://agupubs.onlinelibrary.wiley.com/doi/10.1029/2021EF002612

Extract

Abstract

Ryan et al. (2022) quantified per-fuel-type pollution emission factors and radiative forcing for the 2019 rocket launch fleet plus space-tourism extrapolations. The paper provides the canonical emission factors per kg propellant burned for kerosene/HTPB, hypergolic, liquid hydrogen, and solid fuels. Contemporary 2019 launches produced +3.9 mW/m² radiative forcing (predominantly from black carbon in the stratosphere). Space-tourism extrapolation over 3 years projects +7.9 mW/m². Black carbon emitted into the stratosphere is approximately 500× more potent per unit mass than ground-source BC (longer residence time + altitude-amplified radiative effect). Ozone depletion contributors at upper stratosphere (60-90°N, ~40 km): NOx from re-entry heating (51%) and chlorine from solid fuels (49%) — roughly evenly split.

Key claims

Propellant NOx (g/kg) H2O (g/kg) BC (g/kg) HCl (g/kg) Al₂O₃ (g/kg)
Kerosene / HTPB 14 300 35
Hypergolic 20 550 4
Liquid hydrogen 33 1,000 0
Solid 3 370 0 4 380
  • methalox-not-in-table: methalox emission factors not explicitly given. Stoichiometric methane combustion gives 0.6 kg CO2 + 0.49 kg H2O per kg propellant (mass balance from CH4 + 2O2 → CO2 + 2H2O).
  • BC-500x-potency: stratospheric BC "approximately 500 times more" climate-potent than surface BC.
  • ozone-loss-contributors: 51% from re-entry NOx, 49% from solid-fuel chlorine (at 60-90°N, ~40 km, upper stratosphere).
  • contemporary-2019-RF: +3.9 mW/m² radiative forcing from 2019 launches.
  • space-tourism-3yr-RF: +7.9 mW/m² after 3 years of space-tourism launch cadence.

Reviewer notes

Tier S, peer-reviewed primary measurement. The emission-factor table is the most-cited canonical reference for propellant-specific atmospheric pollution. Critical for q2's calc: a Starship-dominated future is methalox (closer to LH2 in emission profile minus the higher H2O fraction). Per kg methalox propellant, primary stratospheric emissions are ~500 g H2O + ~600 g CO2 + ~10 g NOx (less than kerosene's NOx); essentially zero BC, zero Cl, zero alumina. This makes methalox dramatically lower-impact per kg propellant than the current fuel mix Revell 2025 modelled. Re-entry NOx contribution (51% of ozone loss per Ryan 2022) is propellant-independent — it comes from atmospheric N2 dissociation during reentry heating, not from the propellant itself. Even a fully-reusable methalox Starship still produces re-entry NOx during stage descent.